講演情報

[10p-PB3-40]Exceeding 100% tunnel magnetoresistance in perpendicular magnetic tunnel junctions with cubic GaNx barrier

〇(P)Deepak Kumar1, H Kwon1,2, K Suzuki1,2, S Takaoka1,2, S Miki1, S Mizukami1,3 (1.WPI-AIMR Tohoku Univ., 2.Grad. Sch. Eng., Tohoku Univ., 3.CSIS Tohoku Univ.)

キーワード:

Magnetic Tunnel Junction、、Semiconductor、magnetic materials

Magnetic tunnel junctions (MTJs) are key components in spintronic devices, including hard disk drive (HDD) read heads and magnetic random-access memory (MRAM). Conventional MTJs typically employ CoFeB electrodes and an MgO tunnel barrier; however, alternative materials are actively being investigated to enhance device performance. Although MgO-based MTJs exhibit high tunnel magnetoresistance (TMR), they often have high resistance–area (RA) products due to the large MgO bandgap (7.8 eV). Therefore, there is a growing demand for new tunnel barrier materials that can simultaneously provide high TMR ratios and low resistance. Promising candidates include cubic wide-bandgap oxide semiconductors that can epitaxially grow on the (001) planes of ferromagnetic electrodes. In this study, we investigate metastable cubic-GaN, a wide-bandgap semiconductor with a bandgap of ~3eV, as a tunnel barrier material in perpendicular magnetic tunnel junctions (p-MTJs). The MTJ stacks were deposited on a single-crystal MgO(100) substrate using an ultrahigh-vacuum DC/RF magnetron sputtering system with a base pressure below 5E-7Pa. The stacking structures was substrate/Cr(40)/MnGa(30)/Mg(0.4)/CoMnFe(1.3)/Mg(0.5)/MgO(t)/GaN(0.9)/MgO(1)/CoFeB(1.4)/Ta(3)/Ru(5) (thickness is in nm). Transport measurements were performed using the standard four-probe method at 300K. Figure 1 shows a hysteresis loop for the TMR effect in p-MTJ with a 1 nm bottom MgO layer in the barrier, measured at 300K after annealing at Ta = 300°C. We observed perpendicular magnetization for the top CoFeB layer, indicating that perpendicular magnetic anisotropy remains stable even in the presence of the GaN layer. The maximum TMR ratio of ~120% was observed for the bottom MgO layer with a thickness of ≥ 1 nm in the barrier. We also observed that the resistance-area product (RPA) decreased upon introducing a GaN barrier layer, possibly due to a reduction in barrier height.