Presentation Information

[20p-D902-6]Evaluation of Nonlinear Optical Response using Circularly Polarized Light in Chiral Layered Halide Perovskite Thin Films.

〇Daichi Okada1, Fumito Araoka1 (1.RIKEN CEMS)

Keywords:

Chirality,Nonlinear optics,Organic-inorganic hybrid perovskite

In this study, we evaluated the anisotropic response of second harmonic generation (SHG) to circularly polarized excitation in two-dimensional layered perovskite thin films incorporating chiral organic cations. As a result, a highly efficient anisotrpic response with a maximum g value of approximately 1.6 was obtained. Furthermore, we reveal the contribution of magnetic interactions in the nonlinear optical processes, which leads to the significant anisotropic response.